Catalysis: An Integrated Approach
This book concentrates on industrially relevant reactions which are catalyzed by heterogeneous and homogeneous catalysts. Homogeneous catalysis by metal complexes is treated jointly with heterogeneous catalysis using metallic and non-metallic solids. In both areas the high degree of sophistication of spectroscopic techniques and theoretical modelling has led to an enormous increase in our understanding at the molecular level. This holds for the kinetics of the reactions and the reactivities of the catalysts, as well as for the syntheses of the catalytic materials. The development of catalysis science since the first edition of this book has necessitated a thorough revision, including special chapters on biocatalysis, catalyst characterization and adsorption methods. The multidisciplinary nature of catalysis is reflected in the choice of a novel combination of basic disciplines which will be refreshing and inspiring to readers.
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PREPARATION OF SUPPORTED CATALYSTS
Experimental Determination of Reaction Kinetics 417
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acid activation energy active sites adsorbed adsorption alcohol aldehyde alkenes alkyl alumina ammonia antibonding application atomic orbitals biocatalysts bond calcination carbenium ions carbon Catal catalyst catalyst particles catalytic cracking Chapter Chem chemical complex compounds concentration conversion coordination coverage desorption developed dissociation electron enzyme equation equilibrium ethene example feedstock fermentation formation formed function gas phase glucose groups heat heterogeneous catalysis homogeneous catalysis hydride hydrocarbons hydroformylation hydrogen hydrolysis hydrotreatment hydroxyl industrial interaction intermediate ions isobutene isomerization isotactic isotherm kinetic layer ligands linear liquid phase material mechanism methanol methyl mixture molecular molecules obtained occur orbitals overall oxidative addition oxygen phosphine polymer polymerization pore pressure propene proton rate expression rate-determining ratio reactant reaction rate reactive reactor reduction rhodium Section selectivity silica solid solution species spectroscopy step structure substrate surface area synthesis temperature valence vanadia Volume zeolite